Imaging electrons and atoms in action

Quantum Microscopy and Dynamics

The focus of our research is to integrate the techniques of attosecond physics, scanning tunneling microscopy and ultrafast Raman spectroscopy to realize a four-dimensional space-time quantum microscope to capture electrons and atoms in action in molecules, two-dimensional materials and superconductors. The four-dimensional microscope is capable of probing matter at fundamental space-time quantum limits. We also pursue experiments on molecules present in the cavity of 'on-chip' nanodevices exploring different regimes of light-matter interaction.
 

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Imaging atomic motion in a single molecule by femtosecond broadband CARS
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Electron oscillations driven by light-pulses in an on-chip nanodevice, comprising of two gold bowtie nanoatnennas were measured directly in time by using the self-referencing technique of optical homodyne beating.

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Imaging electronic motion in molecules.
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Ultimate stability of vibration, temperature and humidity in the Precision Laboratory of MPI-Stuttgart

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Two-cycle long phase stable laser pulses shine junction of an STM
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Group members (Sept. 2024)
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Tracking electron oscillations in an ”on-chip” quantum nanodevice.
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By tuning the wavelength of the exciting laser it is possible to selectively excite vibrational modes in a single molecule. On interaction with a red-laser, motion of the nitrogen atoms is activated (bottom-inset), whereas on interaction with an orange-laser, the motion of Hydrogen atoms in a single free base phthalocyanine molecule is activated (top-inset)
 

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